Quantum transport through a DNA wire in a dissipative environment

Gutiérrez, Rafael and Mandal, S. and Cuniberti, Gianaurelio (2005) Quantum transport through a DNA wire in a dissipative environment. Nano Letters 5 (6), pp. 1093-1097.

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Other URL: http://dx.doi.org/10.1021/nl050623g

Abstract

Electronic transport through DNA wires in the presence of a strong dissipative environment is investigated. We show that new bath-induced electronic states are formed within the band gap. These states show up in the linear conductance spectrum as a temperature dependent background and lead to a crossover from tunneling to thermal activated behavior with increasing temperature. Depending on the strength of the electron-bath coupling, the conductance at the Fermi level can show a weak exponential or even an algebraic length dependence. Our results suggest a new environmentally induced transport mechanism. This might be relevant for the understanding of molecular conduction experiments in liquid solution, such as those recently performed on poly(GC) oligomers in a water buffer (B. Xu et al., $\lt$I>Nano Lett$\lt$/I>. $\lt$B>2004$\lt$/B>,$\lt$I> 4$\lt$/I>, 1105).

Item Type:Article
Institutions: Physics > Institute of Theroretical Physics > Retired Professors > Group Gianaurelio Cuniberti
Projects:EU Grant: DNA-based molecular nanowires, Graduiertenkolleg Nichtlinearität und Nichtgleichgewicht, Volkswagen Stiftung: Molecular Computing
Identification Number:
ValueType
10.1021/nl050623gDOI
cond-mat/0410660arXiv ID
Subjects:500 Science > 530 Physics
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Owner:Redakteur Physik
Deposited On:20 Mar 2007
Last Modified:20 Jul 2011 23:01
Item ID:1750
Owner Only: item control page