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Characterization of the lowest excited states of [Rh(bpy-h₈)n(bpy-d₈)3-n]³⁺ by highly resolved emission and excitation spectra

Humbs, W. ; Yersin, Hartmut



Zusammenfassung

Highly resolved emission, excitation, and resonantly line-narrowed spectra, as well as emission decay properties of [Rh(bpy-h₈)n(bpy-d₈)3-n]³⁺ (n = 0, 2, 3; bpy = 2,2'-bipyridine) doped into [Zn(bpy-h₈)₃](ClO₄)₂ are presented for the first time. [Rh(bpy-h₈)3]³⁺ and [Rh(bpy-d₈)₃]³⁺ exhibit one low-lying triplet T₁ at 22 757±1 and 22 818±1 cm⁻¹, respectively (blue shift 61 cm⁻¹), while ...

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