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Unraveling the flavin-catalyzed photooxidation of benzylic alcohol with transient absorption spectroscopy from sub-pico- to microseconds

Megerle, U. and Wenninger, M. and Kutta, Roger J. and Lechner, Robert and Dick, Bernhard and König, Burkhard and Riedle, E. (2011) Unraveling the flavin-catalyzed photooxidation of benzylic alcohol with transient absorption spectroscopy from sub-pico- to microseconds. Physical Chemistry Chemical Physics : PCCP (13), pp. 8869-8880.

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Abstract

Flavin-mediated photooxidations have been described for applications in synthetic organic chemistry for some time and are claimed to be a route to the use of solar energy. We present a detailed investigation of the involved photophysical and photochemical steps in methoxybenzyl alcohol oxidation on a timescale ranging from sub-picoseconds to tens of microseconds. The results establish the flavin ...

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Item Type:Article
Date:2011
Institutions:Chemistry and Pharmacy > Institut für Organische Chemie > Lehrstuhl Prof. Dr. Burkhard König
Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie
Projects:GRK 1626 Chemische Photokatalyse, SFB 749: Dynamik und Intermediate molekularer Transformationen, GRK 640 Sensory photoreceptors in natural and artificial systems
Identification Number:
ValueType
10.1039/c1cp20190eDOI
Subjects:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Owner: Regina Hoheisel
Deposited On:16 Feb 2011 09:26
Last Modified:27 Aug 2012 12:59
Item ID:19627
Owner Only: item control page
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