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Hydrogen-Bond Dynamics in a Protic Ionic Liquid: Evidence of Large-Angle Jumps

Hunger, J. and Sonnleitner, THomas and Liu, Liyuan and Buchner, Richard and Bonn, M. and Bakker, H.J. (2012) Hydrogen-Bond Dynamics in a Protic Ionic Liquid: Evidence of Large-Angle Jumps. Journal of Physical Chemistry Letters 3 (20), pp. 3034-3038.

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Abstract

We study the mol. rotation of the protic room-temp. ionic liq. ethylammonium nitrate with dielec. relaxation spectroscopy and femtosecond-IR spectroscopy (fs-IR) of the ammonium N-H vibrations. The results suggest that the rotation of ethylammonium ion takes place via large angular jumps. Such nondiffusive reorientational dynamics is unique to strongly hydrogen-bonded liqs. such as water and ...

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Item Type:Article
Date:2012
Institutions:Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry VI - Physical Chemistry (Solution Chemistry) > PD Dr. Richard Buchner
Identification Number:
ValueType
10.1021/jz301334jDOI
Keywords:relaxation spectroscopy
Subjects:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Owner: Georg Berger
Deposited On:19 Oct 2012 06:03
Last Modified:19 Oct 2012 06:03
Item ID:26529
Owner Only: item control page
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