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Synthesis and Thermal Cyclization of an Enediyne-Sulfonamide

Klein, M. and König, B. (2004) Synthesis and Thermal Cyclization of an Enediyne-Sulfonamide. Tetrahedron 60, 1087 - 1092.

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Abstract

The synthesis of an enediyne sulfonamide by alkylidene carbene rearrangement is reported. The compound cyclizes thermally to give the Bergman product, which was prepared independently for comparison. Like other σ-acceptor substituents at the enediyne alkyne termini, such as fluoride, oxonium or ammonium groups, the sulfonamide moiety enhances the reactivity for thermal Bergman cyclization as ...

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Item Type:Article
Date:2004
Institutions:Chemistry and Pharmacy > Institut für Organische Chemie > Lehrstuhl Prof. Dr. Burkhard König
Projects:GRK 760, Graduiertenkolleg Medizinische Chemie
Identification Number:
ValueType
10.1016/j.tet.2003.11.078 DOI
Keywords:Enediyne; Yne-amine; Carbene rearrangement; Thermal cyclization
Subjects:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Owner: Regina Hoheisel
Deposited On:05 Mar 2009 10:54
Last Modified:09 Nov 2010 15:36
Item ID:6236
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