Brack, Matthias and Winkler, P and Murthy, N (2008) Coupling of surface and volume dipole oscillations in C-60 molecules. International Journal of Modern Physics E 17, p. 138.
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We first give a short review of the ``local-current approximation'' (LCA), derived from a general variation principle, which serves as a semiclassical description of strongly collective excitations in finite fermion systems starting from their quantum-mechanical mean-field ground state. We illustrate it for the example of coupled translational and compressional dipole excitations in metal clusters. We then discuss collective electronic dipole excitations in C molecules (Buckminster fullerenes). We show that the coupling of the pure translational mode (``surface plasmon'') with compressional volume modes in the semiclasscial LCA yields semi-quantitative agreement with microscopic time-dependent density functional (TDLDA) calculations, while both theories yield qualitative agreement with the recent experimental observation of a ``volume plasmon''.
|Institutions:||Physics > Institute of Theroretical Physics > Chair Professor Schäfer > Group Matthias Brack|
|Projects:||Graduiertenkolleg Nichtlinearität und Nichtgleichgewicht|
|Subjects:||500 Science > 530 Physics|
|Refereed:||Yes, this version has been refereed|
|Created at the University of Regensburg:||Yes|
|Deposited On:||25 May 2009 13:18|
|Last Modified:||05 Aug 2009 13:57|