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Abstract
A sequence consisting of photocatalytic hydrogen atom abstraction (HAT), reductive radical‑polar crossover (RRPCO), and protonation/deuteration for stereochemical editing at benzylic positions is described. A systematic screening of substrates with benzylic C‑H bonds provides trends in reactivity for C‑H activation by silane thiols. A cis/trans isomerization of dihydrobenzofurans proceeding under ...
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