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The First PH-Functionalized Polyphosphazene: A Liquid Macromolecule with Highly Flexible Backbone

Raab, M. ; Schick, G. ; Fondermann, M. D. ; Henze, W. ; Weymand, U. ; Gschwind, R. M. ; Fischer, K. ; Schmidt, M. ; Niecke, E.


The simplest side group: The first example of a completely H-substituted polyphosphazene I is obtained by the polycondensation of (Me2N)2PNH2 in solution at low temperature. NMR investigations and light-scattering experiments substantiate the constitution of the polymer. The conformation and a reaction pathway to I are proposed on the basis of ab initio calculations.

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