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Optically detected magnetic resonance in the lowest triplet state of Pd(2-thpy)₂

Glasbeek, M. ; Sitters, R. ; van Veldhoven, E. ; von Zelewsky, A. ; Humbs, W. ; Yersin, Hartmut


An optically detected magnetic resonance (ODMR) study of the lowest excited state of Pd(2-thpy)₂ ((2-thpy)⁻ = 2-thienylpyridinate) in an n-octane Shpol’skii matrix at T = 1.4 K is reported. The results in zero and low magnetic fields allow us to characterize the emissive triplet state in more detail. In this state the spin-orbit contributions to the zero-field splittings of the triplet substates ...


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