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Rattling the cage: Micro- to mesoscopic structure in liquids as simple as argon and as complicated as water

Turton, D.A. ; Hunger, J. ; Stoppa, A. ; Thoman, A. ; Candelaresi, G. ; Hefter, Glenn ; Walther, M. ; Buchner, Richard ; Wynne, K.


A review. The water mol. has the convenient property that its mol. polarizability tensor is nearly isotropic while its dipole moment is large. As a result, the low-frequency anisotropic Raman spectrum of liq. water is mostly collision-induced and therefore reports primarily translational motions while the far-IR (terahertz) and dielec. spectrum is dominated by rotational modes. Atomic and ...


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