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Dynamic Solvent Effects in Electrochemical Kinetics: Indications for a Switch of the Relevant Solvent Mode

Zagrebin, P.A. ; Buchner, Richard ; Nazmutdinov, R.R. ; Tsirlina, G.A.


The influence of solvent dielec. relaxation on the rate of electron transfer (ET) at an electrochem. interface is addressed using both expt. and model calcns. H2O-ethylene glycol (EG) mixts. were chosen as the solvent because their optical permittivity remains practically const. over the entire compn. range. This allows observation of the dynamic solvent effect with a very minor interference ...


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