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Enhanced Photocatalytic Hydrogen Production by Adsorption of an [FeFe]-Hydrogenase Subunit Mimic on Self-Assembled

Troppmann, Stefan ; Brandes, Eva ; Motschmann, Hubert ; Li, Fei ; Wang, Mei ; Sun, Licheng ; König, Burkhard


Self-assembled vesicles with membrane-embedded or adsorbed ruthenium polypyridine complexes were further functionalized by the adsorption of an [FeFe]-hydrogenase subunit mimic to the membrane interface enhancing the photocatalytic hydrogen production in water under acidic conditions. The resulting two-dimensional membrane assembly places the photosensitizer and hydrogen-evolving diiron complex ...


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