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Atom-Economic Electron Donors for Photobiocatalytic Halogenations

Seel, Catharina Julia ; Králík, Antonin ; Hacker, Melanie ; Frank, Anna ; König, Burkhard ; Gulder, Tanja



Abstract

In vitro cofactor supply and regeneration have been a major obstacle for biocatalytic processes, in particular on a large scale. Peroxidases often suffer from inactivation by their oxidative co-factor. Combining photocatalysis and biocatalysis offers an innovative solution to this problem, but lacks atom economy due to the sacrificial electron donors needed. Herein, we show that redox-active ...

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