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Mooshammer, Fabian ; Sandner, Fabian ; Huber, Markus A. ; Zizlsperger, Martin ; Weigand, Helena ; Plankl, Markus ; Weyrich, Christian ; Lanius, Martin ; Kampmeier, Jörn ; Mussler, G. ; Grützmacher, D. ; Boland, Jessica L. ; Cocker, Tyler L. ; Huber, Rupert

Nanoscale Near-Field Tomography of Surface States on (Bi0.5Sb0.5)2Te3

Mooshammer, Fabian , Sandner, Fabian, Huber, Markus A. , Zizlsperger, Martin, Weigand, Helena, Plankl, Markus, Weyrich, Christian, Lanius, Martin, Kampmeier, Jörn, Mussler, G., Grützmacher, D., Boland, Jessica L. , Cocker, Tyler L. und Huber, Rupert (2018) Nanoscale Near-Field Tomography of Surface States on (Bi0.5Sb0.5)2Te3. Nano Letters 18 (12), S. 7515-7523.

Veröffentlichungsdatum dieses Volltextes: 22 Nov 2018 09:36
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.38043


Zusammenfassung

Three-dimensional topological insulators (TIs) have attracted tremendous interest for their possibility to host massless Dirac Fermions in topologically protected surface states (TSSs), which may enable new kinds of high-speed electronics. However, recent reports have outlined the importance of band bending effects within these materials, which results in an additional two-dimensional electron ...

Three-dimensional topological insulators (TIs) have attracted tremendous interest for their possibility to host massless Dirac Fermions in topologically protected surface states (TSSs), which may enable new kinds of high-speed electronics. However, recent reports have outlined the importance of band bending effects within these materials, which results in an additional two-dimensional electron gas (2DEG) with finite mass at the surface. TI surfaces are also known to be highly inhomogeneous on the nanoscale, which is masked in conventional far-field studies. Here, we use near-field microscopy in the mid infrared spectral range to probe the local surface properties of customtailored (Bi0.5Sb0.5)(2)Te-3 structures with nanometer precision in all three spatial dimensions. Applying nanotomography and nanospectroscopy, we reveal a few-nanometer-thick layer of high surface conductivity and retrieve its local dielectric function without assuming any model for the spectral response. This allows us to directly distinguish between different types of surface states. An intersubband transition within the massive 2DEG formed by quantum confinement in the bent conduction band manifests itself as a sharp, surface-bound, Lorentzian-shaped resonance. An additional broadband background in the imaginary part of the dielectric function may be caused by the TSS. Tracing the intersubband resonance with nanometer spatial precision, we observe changes of its frequency, likely originating from local variations of doping or/and the mixing ratio between Bi and Sb. Our results highlight the importance of studying the surfaces of these novel materials on the nanoscale to directly access the local optical and electronic properties via the dielectric function.



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    Vorschau
    Mooshammer, Fabian , Sandner, Fabian, Huber, Markus A. , Zizlsperger, Martin, Weigand, Helena, Plankl, Markus, Weyrich, Christian, Lanius, Martin, Kampmeier, Jörn, Mussler, G., Grützmacher, D., Boland, Jessica L. , Cocker, Tyler L. und Huber, Rupert (2018) Nanoscale Near-Field Tomography of Surface States on (Bi0.5Sb0.5)2Te3. Nano Letters 18 (12), S. 7515-7523. [Gegenwärtig angezeigt]

Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNano Letters
Verlag:AMER CHEMICAL SOC
Ort der Veröffentlichung:WASHINGTON
Band:18
Nummer des Zeitschriftenheftes oder des Kapitels:12
Seitenbereich:S. 7515-7523
Datum13 November 2018
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1021/acs.nanolett.8b03008DOI
Stichwörter / Keywords3-DIMENSIONAL TOPOLOGICAL INSULATOR; ANALYTICAL-MODEL; DIRAC PLASMONS; FLOQUET-BLOCH; SCATTERING; BI2TE3; SB2TE3; BI2SE3; PHOTOCURRENTS; SPECTROSCOPY; Near-field microscopy; SNOM; tomography; topological insulator; surface state; band bending
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-380436
Dokumenten-ID38043

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