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Puchert, Robin P. ; Steiner, Florian ; Plechinger, Gerd ; Hofmann, Felix J. ; Caspers, Ines ; Kirschner, Johanna ; Nagler, Philipp ; Chernikov, Alexey ; Schüller, Christian ; Korn, Tobias ; Vogelsang, Jan ; Bange, Sebastian ; Lupton, John M.

Spectral focusing of broadband silver electroluminescence in nanoscopic FRET-LEDs

Puchert, Robin P., Steiner, Florian, Plechinger, Gerd , Hofmann, Felix J., Caspers, Ines, Kirschner, Johanna, Nagler, Philipp, Chernikov, Alexey, Schüller, Christian, Korn, Tobias , Vogelsang, Jan , Bange, Sebastian and Lupton, John M. (2017) Spectral focusing of broadband silver electroluminescence in nanoscopic FRET-LEDs. Nature Nanotechnology 12, pp. 637-641.

Date of publication of this fulltext: 14 Mar 2019 08:40
Article
DOI to cite this document: 10.5283/epub.38434


Abstract

Few inventions have shaped the world like the incandescent bulb. Edison used thermal radiation from ohmically heated conductors, but some noble metals also exhibit ‘cold’ electroluminescence in percolation films1,2, tunnel diodes3, electromigrated nanoparticle aggregates4,5, optical antennas6 or scanning tunnelling microscopy7,8,9. The origin of this radiation, which is spectrally broad and ...

Few inventions have shaped the world like the incandescent bulb. Edison used thermal radiation from ohmically heated conductors, but some noble metals also exhibit ‘cold’ electroluminescence in percolation films1,2, tunnel diodes3, electromigrated nanoparticle aggregates4,5, optical antennas6 or scanning tunnelling microscopy7,8,9. The origin of this radiation, which is spectrally broad and depends on applied bias, is controversial given the low radiative yields of electronic transitions. Nanoparticle electroluminescence is particularly intriguing because it involves localized surface-plasmon resonances with large dipole moments. Such plasmons enable very efficient non-radiative fluorescence resonance energy transfer (FRET) coupling to proximal resonant dipole transitions. Here, we demonstrate nanoscopic FRET–light-emitting diodes which exploit the opposite process, energy transfer from silver nanoparticles to exfoliated monolayers of transition-metal dichalcogenides10. In diffraction-limited hotspots showing pronounced photon bunching, broadband silver electroluminescence is focused into the narrow excitonic resonance of the atomically thin overlayer. Such devices may offer alternatives to conventional nano-light-emitting diodes11 in on-chip optical interconnects.



Involved Institutions


Details

Item typeArticle
Journal or Publication TitleNature Nanotechnology
Publisher:Springer
Volume:12
Page Range:pp. 637-641
Date2017
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group Christian Schüller
Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton
Identification Number
ValueType
10.1038/nnano.2017.48DOI
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-384343
Item ID38434

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