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Spectral focusing of broadband silver electroluminescence in nanoscopic FRET-LEDs
Puchert, Robin P., Steiner, Florian, Plechinger, Gerd
, Hofmann, Felix J., Caspers, Ines, Kirschner, Johanna, Nagler, Philipp, Chernikov, Alexey, Schüller, Christian, Korn, Tobias
, Vogelsang, Jan
, Bange, Sebastian
and Lupton, John M.
(2017)
Spectral focusing of broadband silver electroluminescence in nanoscopic FRET-LEDs.
Nature Nanotechnology 12, pp. 637-641.
Date of publication of this fulltext: 14 Mar 2019 08:40
Article
DOI to cite this document: 10.5283/epub.38434
Abstract
Few inventions have shaped the world like the incandescent bulb. Edison used thermal radiation from ohmically heated conductors, but some noble metals also exhibit ‘cold’ electroluminescence in percolation films1,2, tunnel diodes3, electromigrated nanoparticle aggregates4,5, optical antennas6 or scanning tunnelling microscopy7,8,9. The origin of this radiation, which is spectrally broad and ...
Few inventions have shaped the world like the incandescent bulb. Edison used thermal radiation from ohmically heated conductors, but some noble metals also exhibit ‘cold’ electroluminescence in percolation films1,2, tunnel diodes3, electromigrated nanoparticle aggregates4,5, optical antennas6 or scanning tunnelling microscopy7,8,9. The origin of this radiation, which is spectrally broad and depends on applied bias, is controversial given the low radiative yields of electronic transitions. Nanoparticle electroluminescence is particularly intriguing because it involves localized surface-plasmon resonances with large dipole moments. Such plasmons enable very efficient non-radiative fluorescence resonance energy transfer (FRET) coupling to proximal resonant dipole transitions. Here, we demonstrate nanoscopic FRET–light-emitting diodes which exploit the opposite process, energy transfer from silver nanoparticles to exfoliated monolayers of transition-metal dichalcogenides10. In diffraction-limited hotspots showing pronounced photon bunching, broadband silver electroluminescence is focused into the narrow excitonic resonance of the atomically thin overlayer. Such devices may offer alternatives to conventional nano-light-emitting diodes11 in on-chip optical interconnects.
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| Item type | Article | ||||
| Journal or Publication Title | Nature Nanotechnology | ||||
| Publisher: | Springer | ||||
|---|---|---|---|---|---|
| Volume: | 12 | ||||
| Page Range: | pp. 637-641 | ||||
| Date | 2017 | ||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group Christian Schüller Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton | ||||
| Identification Number |
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| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Yes | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-384343 | ||||
| Item ID | 38434 |
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