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Photoinitiated Carbonyl-Metathesis: Deoxygenative Reductive Olefination of Aromatic Aldehydes via Photoredox Catalysis

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Wang, Shun ; Lokesh, Nanjundappa ; Hioe, Johnny ; Gschwind, Ruth M. ; König, Burkhard
License: Creative Commons: Attribution-Noncommercial 3.0
PDF - Accepted Version
Date of publication of this fulltext: 21 Mar 2019 06:37


Carbonyl-carbonyl olefination, known as McMurry reaction, represents a powerful strategy for the construction of olefins. However, catalytic variants that directly couple two carbonyl groups in a single reaction are less explored. Here, we report a photoredox-catalysis that uses B2Pin2 as terminal reductant and oxygen trap allowing for deoxygenative olefination of aromatic aldehydes under mild ...


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