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Perdeuteration of poly[2-methoxy-5-(2'- ethylhexyloxy)-1,4-phenylenevinylene] (d-MEH-PPV): control of microscopic charge-carrier spin–spin coupling and of magnetic-field effects in optoelectronic devices

Stoltzfus, Dani M. ; Joshi, Gajadhar ; Popli, Henna ; Jamali, Shirin ; Kavand, Marzieh ; Milster, Sebastian ; Grünbaum, Tobias ; Bange, Sebastian ; Nahlawi, Adnan ; Teferi, Mandefro Y. ; Atwood, Sabastian I. ; Leung, Anna E. ; Darwish, Tamim A. ; Malissa, Hans ; Burn, Paul L. ; Lupton, John M. ; Boehme, Christoph
Date of publication of this fulltext: 02 Mar 2020 09:49


Abstract

Control of the effective local hyperfine fields in a conjugated polymer, poly[2-methoxy-5-(2'-ethylhexyloxy)-1,4-phenylenevinylene] (MEH-PPV), by isotopic engineering is reported. These fields, evident as a frequency- independent line broadening mechanism in electrically detected magnetic resonance (EDMR) spectroscopy, originate from the unresolved hyperfine coupling between the electronic spin ...

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