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Hybridized intervalley moiré excitons and flat bands in twisted WSe2 bilayers
Brem, Samuel
, Lin, Kai-Qiang
, Gillen, Roland, Bauer, Jonas, Maultzsch, Janina
, Lupton, John M.
and Malic, Ermin
(2020)
Hybridized intervalley moiré excitons and flat bands in twisted WSe2 bilayers.
Nanoscale 12, p. 11088.
Date of publication of this fulltext: 08 Oct 2020 07:54
Article
DOI to cite this document: 10.5283/epub.43868
Abstract
The large surface-to-volume ratio in atomically thin 2D materials allows to efficiently tune their properties through modifications of their environment. Artificial stacking of two monolayers into a bilayer leads to an overlap of layer-localized wave functions giving rise to a twist angle-dependent hybridization of excitonic states. In this joint theory-experiment study, we demonstrate the impact ...
The large surface-to-volume ratio in atomically thin 2D materials allows to efficiently tune their properties through modifications of their environment. Artificial stacking of two monolayers into a bilayer leads to an overlap of layer-localized wave functions giving rise to a twist angle-dependent hybridization of excitonic states. In this joint theory-experiment study, we demonstrate the impact of interlayer hybridization on bright and momentum-dark excitons in twisted WSe2 bilayers. In particular, we show that the strong hybridization of electrons at the Λ point leads to a drastic redshift of the momentum-dark K–Λ exciton, accompanied by the emergence of flat moiré exciton bands at small twist angles. We directly compare theoretically predicted and experimentally measured optical spectra allowing us to identify photoluminescence signals stemming from phonon-assisted recombination of layer-hybridized dark excitons. Moreover, we predict the emergence of additional spectral features resulting from the moiré potential of the twisted bilayer lattice.
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Details
| Item type | Article | ||||
| Journal or Publication Title | Nanoscale | ||||
| Publisher: | Royal Society of Chemistry (RSC) | ||||
|---|---|---|---|---|---|
| Volume: | 12 | ||||
| Page Range: | p. 11088 | ||||
| Date | 17 May 2020 | ||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton | ||||
| Identification Number |
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| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Yes | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-438688 | ||||
| Item ID | 43868 |
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