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Brem, Samuel ; Lin, Kai-Qiang ; Gillen, Roland ; Bauer, Jonas ; Maultzsch, Janina ; Lupton, John M. ; Malic, Ermin

Hybridized intervalley moiré excitons and flat bands in twisted WSe2 bilayers

Brem, Samuel , Lin, Kai-Qiang , Gillen, Roland, Bauer, Jonas, Maultzsch, Janina , Lupton, John M. und Malic, Ermin (2020) Hybridized intervalley moiré excitons and flat bands in twisted WSe2 bilayers. Nanoscale 12, S. 11088.

Veröffentlichungsdatum dieses Volltextes: 08 Okt 2020 07:54
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.43868


Zusammenfassung

The large surface-to-volume ratio in atomically thin 2D materials allows to efficiently tune their properties through modifications of their environment. Artificial stacking of two monolayers into a bilayer leads to an overlap of layer-localized wave functions giving rise to a twist angle-dependent hybridization of excitonic states. In this joint theory-experiment study, we demonstrate the impact ...

The large surface-to-volume ratio in atomically thin 2D materials allows to efficiently tune their properties through modifications of their environment. Artificial stacking of two monolayers into a bilayer leads to an overlap of layer-localized wave functions giving rise to a twist angle-dependent hybridization of excitonic states. In this joint theory-experiment study, we demonstrate the impact of interlayer hybridization on bright and momentum-dark excitons in twisted WSe2 bilayers. In particular, we show that the strong hybridization of electrons at the Λ point leads to a drastic redshift of the momentum-dark K–Λ exciton, accompanied by the emergence of flat moiré exciton bands at small twist angles. We directly compare theoretically predicted and experimentally measured optical spectra allowing us to identify photoluminescence signals stemming from phonon-assisted recombination of layer-hybridized dark excitons. Moreover, we predict the emergence of additional spectral features resulting from the moiré potential of the twisted bilayer lattice.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNanoscale
Verlag:Royal Society of Chemistry (RSC)
Band:12
Seitenbereich:S. 11088
Datum17 Mai 2020
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe John Lupton
Identifikationsnummer
WertTyp
10.1039/D0NR02160ADOI
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-438688
Dokumenten-ID43868

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