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Brem, Samuel ; Lin, Kai-Qiang ; Gillen, Roland ; Bauer, Jonas ; Maultzsch, Janina ; Lupton, John M. ; Malic, Ermin

Hybridized intervalley moiré excitons and flat bands in twisted WSe2 bilayers

Brem, Samuel , Lin, Kai-Qiang , Gillen, Roland, Bauer, Jonas, Maultzsch, Janina , Lupton, John M. and Malic, Ermin (2020) Hybridized intervalley moiré excitons and flat bands in twisted WSe2 bilayers. Nanoscale 12, p. 11088.

Date of publication of this fulltext: 08 Oct 2020 07:54
Article
DOI to cite this document: 10.5283/epub.43868


Abstract

The large surface-to-volume ratio in atomically thin 2D materials allows to efficiently tune their properties through modifications of their environment. Artificial stacking of two monolayers into a bilayer leads to an overlap of layer-localized wave functions giving rise to a twist angle-dependent hybridization of excitonic states. In this joint theory-experiment study, we demonstrate the impact ...

The large surface-to-volume ratio in atomically thin 2D materials allows to efficiently tune their properties through modifications of their environment. Artificial stacking of two monolayers into a bilayer leads to an overlap of layer-localized wave functions giving rise to a twist angle-dependent hybridization of excitonic states. In this joint theory-experiment study, we demonstrate the impact of interlayer hybridization on bright and momentum-dark excitons in twisted WSe2 bilayers. In particular, we show that the strong hybridization of electrons at the Λ point leads to a drastic redshift of the momentum-dark K–Λ exciton, accompanied by the emergence of flat moiré exciton bands at small twist angles. We directly compare theoretically predicted and experimentally measured optical spectra allowing us to identify photoluminescence signals stemming from phonon-assisted recombination of layer-hybridized dark excitons. Moreover, we predict the emergence of additional spectral features resulting from the moiré potential of the twisted bilayer lattice.



Involved Institutions


Details

Item typeArticle
Journal or Publication TitleNanoscale
Publisher:Royal Society of Chemistry (RSC)
Volume:12
Page Range:p. 11088
Date17 May 2020
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton
Identification Number
ValueType
10.1039/D0NR02160ADOI
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-438688
Item ID43868

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