| Accepted Version Download ( PDF | 728kB) | |
Daten und pdf | Data Download ( ZIP Archive | 73MB) Repository staff only |
Measuring the Magnetic Field Amplitude of rf Radiation by the Quasistatic Magnetic Field Effect in Organic Light-Emitting Diodes
Grünbaum, Tobias
, Bange, Sebastian, Jiang, Wei
, Leung, Anna E., Darwish, Tamim A.
, Burn, Paul L.
and Lupton, John M.
(2021)
Measuring the Magnetic Field Amplitude of rf Radiation by the Quasistatic Magnetic Field Effect in Organic Light-Emitting Diodes.
Physical Review Applied 15 (6), 064001.
Date of publication of this fulltext: 07 Jun 2021 04:36
Article
DOI to cite this document: 10.5283/epub.45919
Abstract
Electron paramagnetic resonance (EPR) is a versatile tool to probe spin physics in organic semiconductor materials. A common method used to detect the spin-%2 paramagnetic resonance in organic light-emitting diodes (OLEDs) is to measure the device resistance under EPR conditions, i.e., to record electrically detected magnetic resonance (EDMR). Here, we present ultralow-frequency EDMR experiments ...
Electron paramagnetic resonance (EPR) is a versatile tool to probe spin physics in organic semiconductor materials. A common method used to detect the spin-%2 paramagnetic resonance in organic light-emitting diodes (OLEDs) is to measure the device resistance under EPR conditions, i.e., to record electrically detected magnetic resonance (EDMR). Here, we present ultralow-frequency EDMR experiments on OLEDs that exhibit a qualitatively new line shape because of a quasistatic magnetic field effect: the modulation of the static ultrasmall field-effect magnetoresistance arising from the magnetic field amplitude B1 of the radio frequency (rf) radiation. The disappearance of spin-%2 Zeeman resonances of individual charge carriers in the OLED, i.e., the resonances at magnetic fields where the Zeeman splitting matches the photon energy of the incident rf radiation, coincides with the emergence of the quasistatic effect. We discuss the origin of this quasistatic magnetic field effect, its characteristic line shape in terms of the magnetic field dependence, the influence of experimental parameters, and the application potential with regards to EDMR experiments. The EDMR line shape can be inferred numerically from the magnetoresistance measurements. This approach enables a unique means of determining the drive-field strength B1 in EDMR under driving conditions where alternative methods employing an analysis of the Zeeman resonance-such as power broadening and Rabi flopping-are not applicable.
Alternative links to fulltext
Involved Institutions
Details
| Item type | Article | ||||
| Journal or Publication Title | Physical Review Applied | ||||
| Publisher: | American Physical Society (APS) | ||||
|---|---|---|---|---|---|
| Open Access Type: | Due to SHERPA/RoMEO | ||||
| Place of Publication: | COLLEGE PK | ||||
| Volume: | 15 | ||||
| Number of Issue or Book Chapter: | 6 | ||||
| Page Range: | 064001 | ||||
| Date | 1 June 2021 | ||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton | ||||
| Projects |
Funded by:
Deutsche Forschungsgemeinschaft (DFG)
(314695032)
| ||||
| Identification Number |
| ||||
| Keywords | ROOM-TEMPERATURE; MAGNETORESISTANCE; POLYMER | ||||
| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Yes | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-459194 | ||||
| Item ID | 45919 |
Download Statistics
Download Statistics