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Isotropic Effective Spin-Orbit Coupling in a Conjugated Polymer

Joshi, Gajadhar ; Teferi, Mandefro Y. ; Miller, Richards ; Jamali, Shirin ; Baird, Douglas ; van Tol, Johan ; Malissa, Hans ; Lupton, John M. ; Boehme, Christoph


Conjugated polymers are anisotropic in shape and with regard to electronic properties. Little is known as to how electronic anisotropy impacts the underlying characteristics of the electron spin, such as the coupling to orbital magnetic moments. Using multi-frequency electrically detected magnetic resonance spectroscopy extending over 12 octaves in frequency, we explore the effect of spin-orbit ...


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