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Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2
Raiber, Simon, Faria Junior, Paulo E., Falter, Dennis, Feldl, Simon, Marzena, Petter, Watanabe, Kenji
, Taniguchi, Takashi, Fabian, Jaroslav
and Schüller, Christian
(2022)
Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2.
Nature Communications 13, art.no.4997.
Date of publication of this fulltext: 30 Aug 2022 06:21
Article
DOI to cite this document: 10.5283/epub.52826
Abstract
Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an ...
Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an extra degree of freedom to their electrons, the so-called valley index or valley pseudospin, which behaves conceptually like the electron spin. Here, we present investigations of excitonic transitions in mono- and multilayer WSe2 and MoSe2 materials by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, B-parallel to, of up to 9 T. In monolayer samples, the measured TRFE time traces are almost independent of B-parallel to, which confirms a close to zero in-plane exciton g factor g(parallel to), consistent with first-principles calculations. In contrast, we observe pronounced temporal oscillations in multilayer samples for B-parallel to > 0. Our first-principles calculations confirm the presence of a non-zero g(parallel to) for the multilayer samples. We propose that the oscillatory TRFE signal in the multilayer samples is caused by pseudospin quantum beats of excitons, which is a manifestation of spin- and pseudospin layer locking in the multilayer samples.
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| Item type | Article | ||||
| Journal or Publication Title | Nature Communications | ||||
| Publisher: | Nature | ||||
|---|---|---|---|---|---|
| Open Access Type: | DEAL (Springer Gold) | ||||
| Place of Publication: | BERLIN | ||||
| Volume: | 13 | ||||
| Page Range: | art.no.4997 | ||||
| Date | 25 August 2022 | ||||
| Institutions | Physics > Institute of Theroretical Physics > Chair Professor Richter > Group Jaroslav Fabian Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group Christian Schüller | ||||
| Identification Number |
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| Keywords | SPIN COHERENCE; MONOLAYER; EXCITONS; EXCITATIONS; DIFFUSION; ELECTRONS; LAYER; | ||||
| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Partially | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-528263 | ||||
| Item ID | 52826 |
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