Direkt zum Inhalt

Owner only: item control page
Raiber, Simon ; Faria Junior, Paulo E. ; Falter, Dennis ; Feldl, Simon ; Marzena, Petter ; Watanabe, Kenji ; Taniguchi, Takashi ; Fabian, Jaroslav ; Schüller, Christian

Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2

Raiber, Simon, Faria Junior, Paulo E., Falter, Dennis, Feldl, Simon, Marzena, Petter, Watanabe, Kenji , Taniguchi, Takashi, Fabian, Jaroslav and Schüller, Christian (2022) Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2. Nature Communications 13, art.no.4997.

Date of publication of this fulltext: 30 Aug 2022 06:21
Article
DOI to cite this document: 10.5283/epub.52826


Abstract

Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an ...

Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an extra degree of freedom to their electrons, the so-called valley index or valley pseudospin, which behaves conceptually like the electron spin. Here, we present investigations of excitonic transitions in mono- and multilayer WSe2 and MoSe2 materials by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, B-parallel to, of up to 9 T. In monolayer samples, the measured TRFE time traces are almost independent of B-parallel to, which confirms a close to zero in-plane exciton g factor g(parallel to), consistent with first-principles calculations. In contrast, we observe pronounced temporal oscillations in multilayer samples for B-parallel to > 0. Our first-principles calculations confirm the presence of a non-zero g(parallel to) for the multilayer samples. We propose that the oscillatory TRFE signal in the multilayer samples is caused by pseudospin quantum beats of excitons, which is a manifestation of spin- and pseudospin layer locking in the multilayer samples.



Involved Institutions


Details

Item typeArticle
Journal or Publication TitleNature Communications
Publisher:Nature
Open Access Type:DEAL (Springer Gold)
Place of Publication:BERLIN
Volume:13
Page Range:art.no.4997
Date25 August 2022
InstitutionsPhysics > Institute of Theroretical Physics > Chair Professor Richter > Group Jaroslav Fabian
Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group Christian Schüller
Identification Number
ValueType
10.1038/s41467-022-32534-3DOI
KeywordsSPIN COHERENCE; MONOLAYER; EXCITONS; EXCITATIONS; DIFFUSION; ELECTRONS; LAYER;
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgPartially
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-528263
Item ID52826

Export bibliographical data

Owner only: item control page

nach oben