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Raiber, Simon ; Faria Junior, Paulo E. ; Falter, Dennis ; Feldl, Simon ; Marzena, Petter ; Watanabe, Kenji ; Taniguchi, Takashi ; Fabian, Jaroslav ; Schüller, Christian

Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2

Raiber, Simon, Faria Junior, Paulo E., Falter, Dennis, Feldl, Simon, Marzena, Petter, Watanabe, Kenji , Taniguchi, Takashi, Fabian, Jaroslav und Schüller, Christian (2022) Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2. Nature Communications 13, art.no.4997.

Veröffentlichungsdatum dieses Volltextes: 30 Aug 2022 06:21
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.52826


Zusammenfassung

Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an ...

Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an extra degree of freedom to their electrons, the so-called valley index or valley pseudospin, which behaves conceptually like the electron spin. Here, we present investigations of excitonic transitions in mono- and multilayer WSe2 and MoSe2 materials by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, B-parallel to, of up to 9 T. In monolayer samples, the measured TRFE time traces are almost independent of B-parallel to, which confirms a close to zero in-plane exciton g factor g(parallel to), consistent with first-principles calculations. In contrast, we observe pronounced temporal oscillations in multilayer samples for B-parallel to > 0. Our first-principles calculations confirm the presence of a non-zero g(parallel to) for the multilayer samples. We propose that the oscillatory TRFE signal in the multilayer samples is caused by pseudospin quantum beats of excitons, which is a manifestation of spin- and pseudospin layer locking in the multilayer samples.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNature Communications
Verlag:Nature
Ort der Veröffentlichung:BERLIN
Band:13
Seitenbereich:art.no.4997
Datum25 August 2022
InstitutionenPhysik > Institut für Theoretische Physik > Lehrstuhl Professor Richter > Arbeitsgruppe Jaroslav Fabian
Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe Christian Schüller
Identifikationsnummer
WertTyp
10.1038/s41467-022-32534-3DOI
Stichwörter / KeywordsSPIN COHERENCE; MONOLAYER; EXCITONS; EXCITATIONS; DIFFUSION; ELECTRONS; LAYER;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-528263
Dokumenten-ID52826

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