Direkt zum Inhalt

Raiber, Simon ; Faria Junior, Paulo E. ; Falter, Dennis ; Feldl, Simon ; Marzena, Petter ; Watanabe, Kenji ; Taniguchi, Takashi ; Fabian, Jaroslav ; Schüller, Christian

Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2

Artikel

Raiber, Simon, Faria Junior, Paulo E., Falter, Dennis, Feldl, Simon, Marzena, Petter, Watanabe, Kenji , Taniguchi, Takashi, Fabian, Jaroslav und Schüller, Christian (2022) Ultrafast pseudospin quantum beats in multilayer WSe2 and MoSe2. Nature Communications 13, art.no.4997.

DOI zum Zitieren dieses Dokuments: 10.5283/epub.52826


Zusammenfassung

Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an ...

Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking. Layered van-der-Waals materials with hexagonal symmetry offer an extra degree of freedom to their electrons, the so-called valley index or valley pseudospin, which behaves conceptually like the electron spin. Here, we present investigations of excitonic transitions in mono- and multilayer WSe2 and MoSe2 materials by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, B-parallel to, of up to 9 T. In monolayer samples, the measured TRFE time traces are almost independent of B-parallel to, which confirms a close to zero in-plane exciton g factor g(parallel to), consistent with first-principles calculations. In contrast, we observe pronounced temporal oscillations in multilayer samples for B-parallel to > 0. Our first-principles calculations confirm the presence of a non-zero g(parallel to) for the multilayer samples. We propose that the oscillatory TRFE signal in the multilayer samples is caused by pseudospin quantum beats of excitons, which is a manifestation of spin- and pseudospin layer locking in the multilayer samples.



Beteiligte Einrichtungen


Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNature Communications
VerlagNature
Open Access ArtDEAL (Springer Gold)
Ort der VeröffentlichungBERLIN
Band13
Seitenbereichart.no.4997
Datum25 August 2022
Veröffentlichungsdatum30 Aug 2022 06:21
InstitutionenPhysik > Institut für Theoretische Physik > Lehrstuhl Professor Richter > Arbeitsgruppe Jaroslav Fabian
Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe Christian Schüller
Identifikationsnummer
WertTyp
10.1038/s41467-022-32534-3DOI
Stichwörter / KeywordsSPIN COHERENCE; MONOLAYER; EXCITONS; EXCITATIONS; DIFFUSION; ELECTRONS; LAYER;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-528263
Dokumenten-ID52826

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