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Electron‐Poor Acridones and Acridiniums as Super Photooxidants in Molecular Photoelectrochemistry by Unusual Mechanisms

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Žurauskas, Jonas ; Boháčová, Soňa ; Wu, Shangze ; Butera, Valeria ; Schmid, Simon ; Domański, Michał ; Slanina, Tomáš ; Barham, Joshua Philip
Date of publication of this fulltext: 21 Sep 2023 10:06

This publication is part of the DEAL contract with Wiley.


Electron-deficient acridones and in situ generated acridinium salts are reported as potent, closed-shell photooxidants that undergo surprising mechanisms. When bridging acyclic triarylamine catalysts with a carbonyl group (acridones), this completely diverts their behavior away from open-shell, radical cationic, ‘beyond diffusion’ photocatalysis to closed-shell, neutral, diffusion-controlled ...


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