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Observation of an anomalous increase in total cross sections with high vibrational excitation in the Li2 (V = 0-21) + Na reactive system

Rubahn, H. G. ; Slenczka, A. ; Toennies, J. P.


The effect of initial vibrational excitation on Li2(n,J) + Na collisions was studied exptl. and theor. The relative integral cross sections s(n,J) were measured in a crossed beam expt. for vibrational states n populated thermally or by optical pumping, and for final states detected by laser induced fluorescence. It is found that s(n,J) increases by 35 +- 7% between n = 0 and n = 20, while the ...


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