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Photooxidation of Benzyl Alcohols with Immobilized Flavins

Schmaderer, Harald ; Hilgers, Petra ; Lechner, Robert ; König, Burkhard



Abstract

Benzyl alcohols are oxidized cleanly and efficiently to the corresponding aldehydes under irradiation using flavin photocatalysts and aerial oxygen as the terminal oxidant in homogeneous aqueous solution. Turnover frequencies (TOF) of more than 800 h⁻¹ and turnover numbers (TON) of up to 68 were obtained. Several flavin photocatalysts with fluorinated or hydrophobic aliphatic chains were ...

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