Gierulski, A. and Noda, M. and Yamamoto, T. and Marowsky, G. and Slenczka, A. (1987) Pump-induced population changes in broadband coherent anti-Stokes Raman scattering. Optics Letters 12 (8), pp. 608-10.
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Bu using a powerful, excimer-laser-pumped broadband CARS system, considerable changes were obsd. in the populations of room-temp. N2 under atm. pressure. Pump-induced populations in the 1st, 2nd, and 3rd vibronic bands of N2 at room temp. resulted in an apparent vibrational temp. of 2550 K. The implications for broadband N2 CARS thermometry are discussed.
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|Additional Information (public):||CAN 107:123571; 73-3; Optical, Electron, and Mass Spectroscopy and Other Related Properties; 7727-37-9 (Nitrogen) Role: PRP (Properties) (pump induced population changes in broadband CARS of, temp. detn. in relation to)|
|Institutions:||Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry III - Physical Chemistry (Light and Matter) > Prof. Dr. Alkwin Slenczka|
|Keywords:||Temperature (detn. of, CARS of nitrogen in); Raman spectrometry (CARS, in temp. detn.); CARS nitrogen thermometry; Raman nitrogen thermometry|
|Subjects:||500 Science > 530 Physics|
500 Science > 540 Chemistry & allied sciences
|Refereed:||Yes, this version has been refereed|
|Created at the University of Regensburg:||No|
|Deposited On:||10 Mar 2009 12:48|
|Last Modified:||05 Aug 2009 13:51|