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Organometallic and Classical Coordination Sites in Highly Preorganized Pyrazolate-Based Hybrid Systems: The Mn/Ni Case

Zhang, H. ; Dechert, S. ; Linseis, M. ; Winter, Rainer F. ; Meyer, F.



Abstract

A series of unsymmetric heterodinuclear Mn/Ni complexes is reported in which an organometallic CpMn(CO)(2) fragment and a classical Werner-type nickel(II) subunit are arranged in close proximity by means of a bridging pyrazolate. The two metalloligand scaffolds (1 and 2) employed differ in the chelate size of the tripodal tetradentate (N-4) binding site for nickel. Molecular structures have been ...

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