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Triplets sublevels of metal organic complexes. Temperature dependence of spin-lattice relaxation

Strasser, J. ; Homeier, H. H. H. ; Yersin, Hartmut


Triplets of transition metal complexes with organic chelate ligands can act as important pathways in photo-redox processes. Detailed information on these states is available from highly resolved optical spectra and time-resolved investigations. The lowest triplets are often zero-field split into sublevels by several cm⁻¹ (zero-field splitting, ZFS) due to spin-orbit interactions. Interestingly, ...


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