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Matrix deuteration effects and spin-lattice relaxation in the lowest triplet of the palladium(II)-complex Pd(2-thpy)₂

Becker, D. ; Yersin, Hartmut ; v. Zelewsky, A.


Abstract

Pd(2-thpy)₂ isolated in protonated or deuterated frozen n-octane (Shpol'skii matrices) exhibits highly resolved triplet emission and excitation spectra. One observes interesting differences for the two matrices: (i) The protonated matrix shows only one dominant guest site while the deuterated matrix exhibits two dominant sites. (ii) Low-energy satellites corresponding to lattice modes are ...

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