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Osmotic coefficients and surface tensions of aqueous electrolyte solutions: Role of dispersion forces

Kunz, Werner ; Belloni, L. ; Bernard, Olivier ; Ninham, Barry W.



Abstract

Osmotic coefficients of a series of 16 aqueous electrolyte solutions are described at concentrations up to about 1 M with the help of HNC calculations and solvent-averaged potentials of charged hard spheres with an additional necessary dispersion potential, omitted from all earlier treatments. The adjusted ionic radii and excess polarizabilities have values of the expected order of magnitude. ...

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