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Osmotic coefficients and surface tensions of aqueous electrolyte solutions: Role of dispersion forces

Kunz, Werner ; Belloni, L. ; Bernard, Olivier ; Ninham, Barry W.


Osmotic coeffs. of a series of 16 aq. electrolyte solns. are described at concns. ≤1 M with the help of HNC calcns. and solvent-averaged potentials of charged hard spheres with an addnl. necessary dispersion potential, omitted from all earlier treatments. The adjusted ionic radii and excess polarizabilities have values of the expected order of magnitude. Whereas the description of the bulk ...


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