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Influence of Concentration and Temperature on the Dynamics of Water in the Hydrophobic Hydration Shell of Tetramethylurea

Tielrooij, K.-J. ; Hunger, J. ; Hefter, Glenn ; Buchner, Richard ; Bonn, M. ; Bakker, H.J.


We study the influence of the amphipilic compd. tetramethylurea (TMU) on the dynamical properties of water, using dielec. relaxation spectroscopy in the regime between 0.2 GHz and 2 THz. This technique is capable of resolving different water species, their relative fractions, and their corresponding reorientation dynamics. We find that the reorientation dynamics of water mols. in the hydration ...


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