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Dielectric Spectroscopy of Hydrogen Bond Dynamics and Microheterogenity of Water + Dioxane Mixtures

Schrödle, S. ; Hefter, Glenn ; Buchner, Richard


Mixts. of water or D2O + 1,4-dioxane (DX) have been studied at 25 °C by dielec. relaxation spectroscopy over a wide range of frequencies (0.2 ≤ ν/GHz ≤ 89) for DX mole fractions 0 ≤ x2 ≤ 0.67. The spectra were best fitted by the sum of two Debye terms. The slower process was assigned to the cooperative relaxation of the hydrogen-bond network of water, whereas the faster mode reflects the ...


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