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Coherent electron–nuclear coupling in oligothiophene molecular wires

Repp, Jascha ; Liljeroth, Peter ; Meyer, Gerhard



Abstract

In molecular electronics individual molecules serve as electronic devices. In these systems, electron–vibron (e–ν) coupling can be expected to lead to new physical phenomena and potential device functions1, 2, 3. In previous studies of molecular wires, the e–ν coupling occurred as a result of the well-known Franck–Condon principle, for which the Born–Oppenheimer approximation holds. This means ...

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