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Absence of Singlet Fission and Carrier Multiplication in a Model Conjugated Polymer: Tracking the Triplet Population through Phosphorescence

Bange, Sebastian ; Scherf, Ulrich ; Lupton, John M.


Singlet fission, or multiple exciton generation, has been purported to occur in a variety of material systems. Given the current interest in exploiting this process in photovoltaics, we search for the direct signature of singlet fission, phosphorescence from the triplet state, in a model polymeric organic semiconductor for which photoinduced absorption experiments have implied a tripling of the ...


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