| Veröffentlichte Version Download ( PDF | 1MB) |
Differentiation between polaron-pair and triplet-exciton polaron spin-dependent mechanisms in organic light-emitting diodes by coherent spin beating
Baker, W. J., McCamey, D. R.
, van Schooten, K. J., Lupton, J. M. und make_name_string expected hash reference
(2011)
Differentiation between polaron-pair and triplet-exciton polaron spin-dependent mechanisms in organic light-emitting diodes by coherent spin beating.
Physical Review B (PRB) 84 (16), S. 165205.
Veröffentlichungsdatum dieses Volltextes: 15 Nov 2012 08:21
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.26708
Zusammenfassung
Pulsed electrically detected magnetic resonance offers a unique avenue to distinguish between polaron-pair (PP) and triplet-exciton polaron (TEP) spin-dependent recombination, which control the conductivity and magnetoresistivity of organic semiconductors. Which of these two fundamental processes dominates depends on carrier balance: by injecting surplus electrons we show that both processes ...
Pulsed electrically detected magnetic resonance offers a unique avenue to distinguish between polaron-pair (PP) and triplet-exciton polaron (TEP) spin-dependent recombination, which control the conductivity and magnetoresistivity of organic semiconductors. Which of these two fundamental processes dominates depends on carrier balance: by injecting surplus electrons we show that both processes simultaneously impact the device conductivity. The two mechanisms are distinguished by the presence of a half-field resonance, indicative of TEP interactions, and transient spin beating, the signature of PPs. Coherent spin Rabi flopping in the half-field (triplet) channel is observed, demonstrating that the triplet exciton has an ensemble phase coherence time of at least 60 ns, offering insight into the effect of carrier correlations on spin dephasing.
Alternative Links zum Volltext
Beteiligte Einrichtungen
Details
| Dokumentenart | Artikel | ||||||
| Titel eines Journals oder einer Zeitschrift | Physical Review B (PRB) | ||||||
| Verlag: | AMER PHYSICAL SOC | ||||||
|---|---|---|---|---|---|---|---|
| Ort der Veröffentlichung: | COLLEGE PK | ||||||
| Band: | 84 | ||||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 16 | ||||||
| Seitenbereich: | S. 165205 | ||||||
| Datum | 19 Oktober 2011 | ||||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe John Lupton | ||||||
| Identifikationsnummer |
| ||||||
| Klassifikation |
| ||||||
| Stichwörter / Keywords | PI-CONJUGATED POLYMERS; SEMICONDUCTORS; PHOTOGENERATION; RECOMBINATION; SINGLET; FILMS; | ||||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||||
| Status | Veröffentlicht | ||||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||||
| An der Universität Regensburg entstanden | Zum Teil | ||||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-267086 | ||||||
| Dokumenten-ID | 26708 |
Downloadstatistik
Downloadstatistik