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Fluctuating exciton localization in giant π-conjugated spoked-wheel macrocycles

Agarwal, A. Vikas ; Thiessen, Alexander ; Idelson, Alissa ; Kalle, Daniel ; Würsch, Dominik ; Stangl, Thomas ; Steiner, Florian ; Jester, Stefan-S. ; Vogelsang, Jan ; Höger, Sigurd ; Lupton, John M.



Abstract

Conjugated polymers offer potential for many diverse applications, but we still lack a fundamental microscopic understanding of their electronic structure. Elementary photoexcitations (excitons) span only a few nanometres of a molecule, which itself can extend over microns, and how their behaviour is affected by molecular dimensions is not immediately obvious. For example, where is the exciton ...

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