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Ultrafast insulator-metal phase transition in VO2 studied by multiterahertz spectroscopy
Pashkin, A., Kübler, C., Ehrke, H., Lopez, R., Halabica, A., Haglund Jr., R. F., Huber, Rupert und Leitenstorfer, A. (2011) Ultrafast insulator-metal phase transition in VO2 studied by multiterahertz spectroscopy. Physical Review B 83, S. 195120.Veröffentlichungsdatum dieses Volltextes: 15 Okt 2014 11:25
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.30886
Zusammenfassung
The ultrafast photoinduced insulator-metal transition in VO2 is studied at different temperatures and excitation fluences using multi-THz probe pulses. The spectrally resolved midinfrared response allows us to trace separately the dynamics of lattice and electronic degrees of freedom with a time resolution of 40 fs. The critical fluence of the optical pump pulse, which drives the system into a ...
The ultrafast photoinduced insulator-metal transition in VO2 is studied at different temperatures and excitation fluences using multi-THz probe pulses. The spectrally resolved midinfrared response allows us to trace separately the dynamics of lattice and electronic degrees of freedom with a time resolution of 40 fs. The critical fluence of the optical pump pulse, which drives the system into a long-lived metallic state, is found to increase with decreasing temperature. Under all measurement conditions, we observe a modulation of the eigenfrequencies of the optical phonon modes induced by their anharmonic coupling to the coherent wave-packet motion of V-V dimers at 6.1 THz. Furthermore, we find a weak quadratic coupling of the electronic response to the coherent dimer oscillation resulting in a modulation of the electronic conductivity at twice the frequency of the wave-packet motion. The findings are discussed in the framework of a qualitative model based on an approximation of local photoexcitation of the vanadium dimers from the insulating state.
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| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Physical Review B | ||||
| Verlag: | American Physical Society | ||||
|---|---|---|---|---|---|
| Band: | 83 | ||||
| Seitenbereich: | S. 195120 | ||||
| Datum | 2011 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber | ||||
| Identifikationsnummer |
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| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Nein | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-308868 | ||||
| Dokumenten-ID | 30886 |
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