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Is surface layering of aqueous alkali halides determined by ion pairing in the bulk solution?

Brandes, Eva ; Stage, Christiane ; Motschmann, Hubert ; Rieder, Julian ; Buchner, Richard


This contribution aims to elucidate the connection between ion-​ion-​solvent interactions in the bulk of aq. electrolyte solns. and the properties of their liq.-​air interface. In particular, we were interested in the conditions under which ion pairs form at the surface and whether this is linked to ion pairing in the bulk. For this reason different combinations of hard (Cl-​, Li+) and soft ...


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