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LED-Illuminated NMR Studies of Flavin-Catalyzed Photooxidations Reveal Solvent Control of the Electron-Transfer Mechanism

Feldmeier, Christian, Bartling, Hanna, Magerl, Kathrin and Gschwind, R. M. (2015) LED-Illuminated NMR Studies of Flavin-Catalyzed Photooxidations Reveal Solvent Control of the Electron-Transfer Mechanism. Angew. Chem. Int. Ed. 54 (4), pp. 1347-1351.

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Abstract

Mechanistic insights into chemical photocatalysis are mainly the domain of UV/Vis spectroscopy, because NMR spectroscopy has been limited by the type of illumination so far. An improved LED-based illumination device can be used to obtain NMR reaction profiles of photocatalytic reactions under synthetic conditions and perform both photo-CIDNP and intermediate studies. Flavin-catalyzed ...

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Item type:Article
Date:19 January 2015
Institutions:Chemistry and Pharmacy > Institut für Organische Chemie > Arbeitskreis Prof. Dr. Ruth Gschwind
Projects:GRK 1626 Chemische Photokatalyse
Identification Number:
ValueType
10.1002/anie.201409146DOI
Keywords:flavin; NMR spectroscopy; photocatalysis; solvent effects; UV/Vis spectroscopy
Dewey Decimal Classification:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Item ID:31251
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