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Ionic Liquids: Not only Structurally but also Dynamically Heterogeneous

Zheng, Zhuan-Ping ; Fan, Wen-Hui ; Roy, Soham ; Mazur, Kamila ; Nazet, Andreas ; Buchner, Richard ; Bonn, Mischa ; Hunger, J.


In recent years, the complex and heterogeneous structure of ionic liqs. was demonstrated; however, the consequences on the dynamics have remained elusive. Here, the authors use femtosecond IR spectroscopy to elucidate the local structural dynamics in protic alkylammonium-based ionic liqs. The structural relaxation after an ultrafast temp. increase, following vibrational excitation and ...


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