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Ionic Liquids: Not only Structurally but also Dynamically Heterogeneous

Zheng, Zhuan-Ping ; Fan, Wen-Hui ; Roy, Soham ; Mazur, Kamila ; Nazet, Andreas ; Buchner, Richard ; Bonn, Mischa ; Hunger, J.



Abstract

In recent years, the complex and heterogeneous structure of ionic liquids has been demonstrated; however, the consequences on the dynamics have remained elusive. Here, we use femtosecond IR spectroscopy to elucidate the local structural dynamics in protic alkylammonium-based ionic liquids. The structural relaxation after an ultrafast temperature increase, following vibrational excitation and ...

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