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Schuler, Bruno ; Persson, Mats ; Paavilainen, Sami ; Pavliček, Niko ; Gross, Leo ; Meyer, Gerhard ; Repp, Jascha

Effect of electron-phonon interaction on the formation of one-dimensional electronic states in coupled Cl vacancies

Article

Schuler, Bruno , Persson, Mats , Paavilainen, Sami , Pavliček, Niko , Gross, Leo , Meyer, Gerhard and Repp, Jascha (2015) Effect of electron-phonon interaction on the formation of one-dimensional electronic states in coupled Cl vacancies. Physical Review B 91, p. 235443.

DOI to cite this document: 10.5283/epub.32012


Abstract

The formation of extended electron states in one-dimensional nanostructures is of key importance for the function of molecular electronic devices. Here, we study the effects of strong electron-phonon interaction on the formation of extended electronic states in intentionally created Cl vacancy pairs and chains in a NaCl bilayer on Cu(111). The interaction between the vacancies was tailored by ...

The formation of extended electron states in one-dimensional nanostructures is of key importance for the function of molecular electronic devices. Here, we study the effects of strong electron-phonon interaction on the formation of extended electronic states in intentionally created Cl vacancy pairs and chains in a NaCl bilayer on Cu(111). The interaction between the vacancies was tailored by fabricating vacancy pairs and chains of different orientation and separation with atomic precision using vertical manipulation. Small vacancy separations led to the formation of quantum-well-like vacancy states and localized interface states. By using scanning tunneling spectroscopy, we measured their energy splitting and broadening as a function of the intervacancy separation. Remarkably, the energy splitting between the vacancy states is enlarged by level repulsion resulting from the phonon dressing of the electronic states, as evidenced by theory.



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Details

Item typeArticle
Journal or Publication TitlePhysical Review B
PublisherAMER PHYSICAL SOC
Open Access TypeDue to SHERPA/RoMEO
Place of PublicationCOLLEGE PK
Volume91
Page Rangep. 235443
Date24 June 2015
Date of publication29 Jun 2015 08:03
InstitutionsPhysics > Institute of Experimental and Applied Physics > Group Jascha Repp
Identification Number
ValueType
10.1103/PhysRevB.91.235443DOI
KeywordsSCANNING TUNNELING MICROSCOPE; QUANTUM DOTS; CHEMICAL-STRUCTURE; FORCE MICROSCOPY; SURFACE; CHAINS; ABSORPTION; SCATTERING; FILMS; WELL;
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgPartially
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-320125
Item ID32012

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