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Effect of electron-phonon interaction on the formation of one-dimensional electronic states in coupled Cl vacancies
Article
Schuler, Bruno
, Persson, Mats
, Paavilainen, Sami
, Pavliček, Niko
, Gross, Leo
, Meyer, Gerhard and Repp, Jascha
(2015)
Effect of electron-phonon interaction on the formation of one-dimensional electronic states in coupled Cl vacancies.
Physical Review B 91, p. 235443.
DOI to cite this document: 10.5283/epub.32012
Abstract
The formation of extended electron states in one-dimensional nanostructures is of key importance for the function of molecular electronic devices. Here, we study the effects of strong electron-phonon interaction on the formation of extended electronic states in intentionally created Cl vacancy pairs and chains in a NaCl bilayer on Cu(111). The interaction between the vacancies was tailored by ...
The formation of extended electron states in one-dimensional nanostructures is of key importance for the function of molecular electronic devices. Here, we study the effects of strong electron-phonon interaction on the formation of extended electronic states in intentionally created Cl vacancy pairs and chains in a NaCl bilayer on Cu(111). The interaction between the vacancies was tailored by fabricating vacancy pairs and chains of different orientation and separation with atomic precision using vertical manipulation. Small vacancy separations led to the formation of quantum-well-like vacancy states and localized interface states. By using scanning tunneling spectroscopy, we measured their energy splitting and broadening as a function of the intervacancy separation. Remarkably, the energy splitting between the vacancy states is enlarged by level repulsion resulting from the phonon dressing of the electronic states, as evidenced by theory.
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Details
| Item type | Article | ||||
| Journal or Publication Title | Physical Review B | ||||
| Publisher | AMER PHYSICAL SOC | ||||
| Open Access Type | Due to SHERPA/RoMEO | ||||
| Place of Publication | COLLEGE PK | ||||
| Volume | 91 | ||||
| Page Range | p. 235443 | ||||
| Date | 24 June 2015 | ||||
| Date of publication | 29 Jun 2015 08:03 | ||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Group Jascha Repp | ||||
| Identification Number |
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| Keywords | SCANNING TUNNELING MICROSCOPE; QUANTUM DOTS; CHEMICAL-STRUCTURE; FORCE MICROSCOPY; SURFACE; CHAINS; ABSORPTION; SCATTERING; FILMS; WELL; | ||||
| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Partially | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-320125 | ||||
| Item ID | 32012 |
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