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Functionalized Vesicles with Co-Embedded CdSe Quantum Dots and [FeFe]-Hydrogenase Mimic for Light-Driven Hydrogen Production

Troppmann, Stefan ; König, Burkhard



Abstract

A photocatalytic hybrid system for the production of hydrogen in purely aqueous solution was prepared by the co-embedding of hydrophobic oleic acid capped CdSe quantum dots (QD) for light harvesting and an amphiphilic [FeFe]-hydrogenase subunit mimic for proton reduction into phospholipid vesicle membranes. These bio-inspired functionalized vesicles concentrate the catalytic subunits in close ...

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