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Raab, Jürgen ; Lange, Christoph ; Boland, Jessica L. ; Laepple, Ignaz ; Furthmeier, Martin ; Dardanis, Enrico ; Dessmann, Nils ; Li, Lianhe ; Linfield, Edmund H. ; Davies, A. Giles ; Vitiello, Miriam S. ; Huber, Rupert

Ultrafast two-dimensional field spectroscopy of terahertz intersubband saturable absorbers

Article

Raab, Jürgen, Lange, Christoph, Boland, Jessica L. , Laepple, Ignaz, Furthmeier, Martin, Dardanis, Enrico, Dessmann, Nils, Li, Lianhe, Linfield, Edmund H., Davies, A. Giles , Vitiello, Miriam S. and Huber, Rupert (2019) Ultrafast two-dimensional field spectroscopy of terahertz intersubband saturable absorbers. Optics Express 27 (3), pp. 2248-2257.

DOI to cite this document: 10.5283/epub.38365


Abstract

Intersubband (ISB) transitions in semiconductor multi-quantum well (MQW) structures are promising candidates for the development of saturable absorbers at terahertz (THz) frequencies. Here, we exploit amplitude and phase-resolved two-dimensional (2D) THz spectroscopy on the sub-cycle time scale to observe directly the saturation dynamics and coherent control of ISB transitions in a ...

Intersubband (ISB) transitions in semiconductor multi-quantum well (MQW) structures are promising candidates for the development of saturable absorbers at terahertz (THz) frequencies. Here, we exploit amplitude and phase-resolved two-dimensional (2D) THz spectroscopy on the sub-cycle time scale to observe directly the saturation dynamics and coherent control of ISB transitions in a metal-insulator MQW structure. Clear signatures of incoherent pump-probe and coherent four-wave mixing signals are recorded as a function of the peak electric field of the single-cycle THz pulses. All nonlinear signals reach a pronounced maximum for a THz electric field amplitude of 11 kV/cm and decrease for higher fields. We demonstrate that this behavior is a fingerprint of THz-driven carrier-wave Rabi flopping. A numerical solution of the Maxwell-Bloch equations reproduces our experimental findings quantitatively and traces the trajectory of the Bloch vector. This microscopic model allows us to design tailored MQW structures with optimized dynamical properties for saturable absorbers that could be used in future compact semiconductor-based single-cycle THz sources. Published by The Optical Society under the terms of the Creative Commons Attribution 4.0 License.



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Details

Item typeArticle
Journal or Publication TitleOptics Express
PublisherOPTICAL SOC AMER
Open Access TypeGold (mit APC - nicht UR)
Place of PublicationWASHINGTON
Volume27
Number of Issue or Book Chapter3
Page Rangepp. 2248-2257
Date25 January 2019
Date of publication18 Feb 2019 12:24
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Identification Number
ValueType
10.1364/OE.27.002248DOI
KeywordsQUANTUM CASCADE LASERS; PULSES; GENERATION; DYNAMICS; RADIATION; EMISSION;
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-383654
Item ID38365

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