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Alkene Metalates as Hydrogenation Catalysts

Büschelberger, Philipp ; Gärtner, Dominik ; Reyes-Rodriguez, Efrain ; Kreyenschmidt, Friedrich ; Koszinowski, Konrad ; Jacobi von Wangelin, Axel ; Wolf, Robert



Abstract

First-row transition-metal complexes hold great potential as catalysts for hydrogenations and related reductive reactions. Homo-and heteroleptic arene/alkene metalates(1-) (M=Co, Fe) are a structurally distinct catalyst class with good activities in hydrogenations of alkenes and alkynes. The first syntheses of the heteroleptic cobaltates [K([18]crown-6)][Co(eta(4)-cod)(eta(2)-styrene)(2)] (5) and ...

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