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Cocker, T. L. ; Baillie, D. ; Buruma, M. ; Titova, L. V. ; Sydora, R. D. ; Marsiglio, F. ; Hegmann, F. A.

Microscopic origin of the Drude-Smith model

Cocker, T. L., Baillie, D., Buruma, M., Titova, L. V., Sydora, R. D., Marsiglio, F. and Hegmann, F. A. (2017) Microscopic origin of the Drude-Smith model. Physical Review B 96 (20).

Date of publication of this fulltext: 20 Mar 2019 13:09
Article
DOI to cite this document: 10.5283/epub.39556


Abstract

The Drude-Smith model has been used extensively in fitting the THz conductivities of nanomaterials with carrier confinement on the mesoscopic scale. Here, we show that the conventional "backscattering" explanation for the suppression of low-frequency conductivities in the Drude-Smith model is not consistent with a confined Drude gas of classical noninteracting electrons and we derive a modified ...

The Drude-Smith model has been used extensively in fitting the THz conductivities of nanomaterials with carrier confinement on the mesoscopic scale. Here, we show that the conventional "backscattering" explanation for the suppression of low-frequency conductivities in the Drude-Smith model is not consistent with a confined Drude gas of classical noninteracting electrons and we derive a modified Drude-Smith conductivity formula based on a diffusive restoring current. We perform Monte Carlo simulations of a model system and show that the modifiedDrude-Smith model reproduces the extracted conductivitieswithout free parameters. This alternate route to the Drude-Smith model provides the popular formula with a more solid physical foundation and well-defined fit parameters.



Involved Institutions


Details

Item typeArticle
Journal or Publication TitlePhysical Review B
Publisher:AMER PHYSICAL SOC
Place of Publication:COLLEGE PK
Volume:96
Number of Issue or Book Chapter:20
Date2017
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Identification Number
ValueType
10.1103/PhysRevB.96.205439DOI
KeywordsRESOLVED TERAHERTZ SPECTROSCOPY; CARRIER DYNAMICS; PROBE SPECTROSCOPY; CHARGE-TRANSPORT; THIN-FILMS; NANOCRYSTAL FILMS; SILICON; CONDUCTIVITY; NANOWIRES; PHOTOCONDUCTIVITY;
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-395566
Item ID39556

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