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Microscopic origin of the Drude-Smith model
Cocker, T. L., Baillie, D., Buruma, M., Titova, L. V., Sydora, R. D., Marsiglio, F. and Hegmann, F. A. (2017) Microscopic origin of the Drude-Smith model. Physical Review B 96 (20).Date of publication of this fulltext: 20 Mar 2019 13:09
Article
DOI to cite this document: 10.5283/epub.39556
Abstract
The Drude-Smith model has been used extensively in fitting the THz conductivities of nanomaterials with carrier confinement on the mesoscopic scale. Here, we show that the conventional "backscattering" explanation for the suppression of low-frequency conductivities in the Drude-Smith model is not consistent with a confined Drude gas of classical noninteracting electrons and we derive a modified ...
The Drude-Smith model has been used extensively in fitting the THz conductivities of nanomaterials with carrier confinement on the mesoscopic scale. Here, we show that the conventional "backscattering" explanation for the suppression of low-frequency conductivities in the Drude-Smith model is not consistent with a confined Drude gas of classical noninteracting electrons and we derive a modified Drude-Smith conductivity formula based on a diffusive restoring current. We perform Monte Carlo simulations of a model system and show that the modifiedDrude-Smith model reproduces the extracted conductivitieswithout free parameters. This alternate route to the Drude-Smith model provides the popular formula with a more solid physical foundation and well-defined fit parameters.
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| Item type | Article | ||||
| Journal or Publication Title | Physical Review B | ||||
| Publisher: | AMER PHYSICAL SOC | ||||
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| Place of Publication: | COLLEGE PK | ||||
| Volume: | 96 | ||||
| Number of Issue or Book Chapter: | 20 | ||||
| Date | 2017 | ||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber | ||||
| Identification Number |
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| Keywords | RESOLVED TERAHERTZ SPECTROSCOPY; CARRIER DYNAMICS; PROBE SPECTROSCOPY; CHARGE-TRANSPORT; THIN-FILMS; NANOCRYSTAL FILMS; SILICON; CONDUCTIVITY; NANOWIRES; PHOTOCONDUCTIVITY; | ||||
| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Yes | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-395566 | ||||
| Item ID | 39556 |
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