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Cocker, T. L. ; Baillie, D. ; Buruma, M. ; Titova, L. V. ; Sydora, R. D. ; Marsiglio, F. ; Hegmann, F. A.

Microscopic origin of the Drude-Smith model

Cocker, T. L., Baillie, D., Buruma, M., Titova, L. V., Sydora, R. D., Marsiglio, F. und Hegmann, F. A. (2017) Microscopic origin of the Drude-Smith model. Physical Review B 96 (20).

Veröffentlichungsdatum dieses Volltextes: 20 Mrz 2019 13:09
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.39556


Zusammenfassung

The Drude-Smith model has been used extensively in fitting the THz conductivities of nanomaterials with carrier confinement on the mesoscopic scale. Here, we show that the conventional "backscattering" explanation for the suppression of low-frequency conductivities in the Drude-Smith model is not consistent with a confined Drude gas of classical noninteracting electrons and we derive a modified ...

The Drude-Smith model has been used extensively in fitting the THz conductivities of nanomaterials with carrier confinement on the mesoscopic scale. Here, we show that the conventional "backscattering" explanation for the suppression of low-frequency conductivities in the Drude-Smith model is not consistent with a confined Drude gas of classical noninteracting electrons and we derive a modified Drude-Smith conductivity formula based on a diffusive restoring current. We perform Monte Carlo simulations of a model system and show that the modifiedDrude-Smith model reproduces the extracted conductivitieswithout free parameters. This alternate route to the Drude-Smith model provides the popular formula with a more solid physical foundation and well-defined fit parameters.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftPhysical Review B
Verlag:AMER PHYSICAL SOC
Ort der Veröffentlichung:COLLEGE PK
Band:96
Nummer des Zeitschriftenheftes oder des Kapitels:20
Datum2017
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1103/PhysRevB.96.205439DOI
Stichwörter / KeywordsRESOLVED TERAHERTZ SPECTROSCOPY; CARRIER DYNAMICS; PROBE SPECTROSCOPY; CHARGE-TRANSPORT; THIN-FILMS; NANOCRYSTAL FILMS; SILICON; CONDUCTIVITY; NANOWIRES; PHOTOCONDUCTIVITY;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-395566
Dokumenten-ID39556

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