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The Role of Electronic and Phononic Excitation in the Optical Response of Monolayer WS2 after Ultrafast Excitation

Ruppert, Claudia ; Chernikov, Alexey ; Hill, Heather M. ; Rigosi, Albert F. ; Heinz, Tony F.



Zusammenfassung

Transient changes of the optical response of WS2 monolayers are studied by femtosecond broadband pump–probe spectroscopy. Time-dependent absorption spectra are analyzed by tracking the line width broadening, bleaching, and energy shift of the main exciton resonance as a function of time delay after the excitation. Two main sources for the pump-induced changes of the optical response are ...

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