| Veröffentlichte Version Download ( PDF | 3MB) |
Exciton Diffusion and Halo Effects in Monolayer Semiconductors
Kulig, Marvin, Zipfel, Jonas, Nagler, Philipp, Blanter, Sofia, Schüller, Christian, Korn, Tobias
, Paradiso, Nicola
, Glazov, Mikhail M.
und Chernikov, Alexey
(2018)
Exciton Diffusion and Halo Effects in Monolayer Semiconductors.
Physical Review Letters 120 (20).
Veröffentlichungsdatum dieses Volltextes: 30 Jul 2019 13:37
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.40601
Zusammenfassung
We directly monitor exciton propagation in freestanding and SiO2-supported WS2 monolayers through spatially and time-resolved microphotoluminescence under ambient conditions. We find a highly nonlinear behavior with characteristic, qualitative changes in the spatial profiles of the exciton emission and an effective diffusion coefficient increasing from 0.3 to more than 30 cm(2)/s, depending on ...
We directly monitor exciton propagation in freestanding and SiO2-supported WS2 monolayers through spatially and time-resolved microphotoluminescence under ambient conditions. We find a highly nonlinear behavior with characteristic, qualitative changes in the spatial profiles of the exciton emission and an effective diffusion coefficient increasing from 0.3 to more than 30 cm(2)/s, depending on the injected exciton density. Solving the diffusion equation while accounting for Auger recombination allows us to identify and quantitatively understand the main origin of the increase in the observed diffusion coefficient. At elevated excitation densities, the initial Gaussian distribution of the excitons evolves into long-lived halo shapes with mu m-scale diameter, indicating additional memory effects in the exciton dynamics.
Alternative Links zum Volltext
Beteiligte Einrichtungen
Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Physical Review Letters | ||||
| Verlag: | AMER PHYSICAL SOC | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | COLLEGE PK | ||||
| Band: | 120 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 20 | ||||
| Datum | 2018 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Entpflichtete oder im Ruhestand befindliche Professoren > Nachwuchsgruppe Alexey Chernikov | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | TRANSPORT; EXCITATION; WSE2; WS2; PHOTOLUMINESCENCE; ELECTRONS; EVOLUTION; DYNAMICS; LIGHT; DECAY; | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-406013 | ||||
| Dokumenten-ID | 40601 |
Downloadstatistik
Downloadstatistik