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Exciton Diffusion and Halo Effects in Monolayer Semiconductors
Kulig, Marvin, Zipfel, Jonas, Nagler, Philipp, Blanter, Sofia, Schüller, Christian, Korn, Tobias
, Paradiso, Nicola
, Glazov, Mikhail M.
and Chernikov, Alexey
(2018)
Exciton Diffusion and Halo Effects in Monolayer Semiconductors.
Physical Review Letters 120 (20).
Date of publication of this fulltext: 30 Jul 2019 13:37
Article
DOI to cite this document: 10.5283/epub.40601
Abstract
We directly monitor exciton propagation in freestanding and SiO2-supported WS2 monolayers through spatially and time-resolved microphotoluminescence under ambient conditions. We find a highly nonlinear behavior with characteristic, qualitative changes in the spatial profiles of the exciton emission and an effective diffusion coefficient increasing from 0.3 to more than 30 cm(2)/s, depending on ...
We directly monitor exciton propagation in freestanding and SiO2-supported WS2 monolayers through spatially and time-resolved microphotoluminescence under ambient conditions. We find a highly nonlinear behavior with characteristic, qualitative changes in the spatial profiles of the exciton emission and an effective diffusion coefficient increasing from 0.3 to more than 30 cm(2)/s, depending on the injected exciton density. Solving the diffusion equation while accounting for Auger recombination allows us to identify and quantitatively understand the main origin of the increase in the observed diffusion coefficient. At elevated excitation densities, the initial Gaussian distribution of the excitons evolves into long-lived halo shapes with mu m-scale diameter, indicating additional memory effects in the exciton dynamics.
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Details
| Item type | Article | ||||
| Journal or Publication Title | Physical Review Letters | ||||
| Publisher: | AMER PHYSICAL SOC | ||||
|---|---|---|---|---|---|
| Place of Publication: | COLLEGE PK | ||||
| Volume: | 120 | ||||
| Number of Issue or Book Chapter: | 20 | ||||
| Date | 2018 | ||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Alumni or Retired Professors > Junior Research Group Alexey Chernikov | ||||
| Identification Number |
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| Keywords | TRANSPORT; EXCITATION; WSE2; WS2; PHOTOLUMINESCENCE; ELECTRONS; EVOLUTION; DYNAMICS; LIGHT; DECAY; | ||||
| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Yes | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-406013 | ||||
| Item ID | 40601 |
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