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Facile C=O Bond Splitting of Carbon Dioxide Induced by Metal-Ligand Cooperativity in a Phosphinine Iron(0) Complex

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Leitl, J. ; Marquardt, M. ; Coburger, Peter ; Scott, D. J. ; Streitferdt, Verena ; Gschwind, R. M. ; Müller, Christian ; Wolf, Robert
License: Creative Commons Attribution Non-commercial 4.0
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Date of publication of this fulltext: 04 Sep 2019 13:20

This publication is part of the DEAL contract with Wiley.


New iron complexes [Cp*FeL](-) (1-sigma and 1-pi, Cp*=C5Me5) containing the chelating phosphinine ligand 2-(2 '-pyridyl)-4,6-diphenylphosphinine (L) have been prepared, and found to undergo facile reaction with CO2 under ambient conditions. The outcome of this reaction depends on the coordination mode of the versatile ligand L. Interaction of CO2 with the isomer 1-pi, in which L binds to Fe ...


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