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Internal Acidity Scale and Reactivity Evaluation of Chiral Phosphoric Acids with different 3,3’-Substituents in Brønsted Acid Catalysis

Rothermel, K. ; Melikian, M. ; Hioe, J. ; Greindl, J, ; Gramüller, J. ; Žabka, M. ; Sorgenfrei, N. ; Hausler, T. ; Morana, F. ; Gschwind, R. M.


The concept of hydrogen bonding for enhancing substrate binding and controlling selectivity and reactivity is central in catalysis. However, the properties of these key hydrogen bonds and their catalyst-dependent variations are extremely difficult to determine directly by experiments. Here, for the first time the hydrogen bond properties of a whole series of BINOL-derived chiral phosphoric acid ...


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