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Disulfonimides Versus Phosphoric Acids in Brønsted Acid Catalysis: The Effect of Weak Hydrogen Bonds and Multiple Acceptors on Complex Structures and Reactivity

Rothermel, K. ; Žabka, M. ; Hioe, J. ; Gschwind, R. M.



Abstract

In Bronsted acid catalysis, hydrogen bonds play a crucial role for reactivity and selectivity. However, the contribution of weak hydrogen bonds or multiple acceptors has been unclear so far since it is extremely difficult to collect experimental evidence for weak hydrogen bonds. Here, our hydrogen bond and structural access to Bronsted acid/imine complexes was used to analyze BINOL-derived chiral ...

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