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Photocatalytic activation of alkyl chlorides by assembly-promoted single electron transfer in microheterogeneous solutions

Giedyk, Maciej, Narobe, Rok, Weiß, Sophia, Touraud, Didier , Kunz, Werner and König, Burkhard (2019) Photocatalytic activation of alkyl chlorides by assembly-promoted single electron transfer in microheterogeneous solutions. Naturecatalysis.

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Other URL: https://www.nature.com/articles/s41929-019-0369-5


Abstract

Photoredox catalysis has developed into a powerful tool for the synthesis of organic compounds with diverse structures. However, stable carbon–chloride bonds remain beyond the energetic limits of the outer-sphere photoreductive activation. Here, we demonstrate that the organization of the reacting species in microstructured, aqueous solutions allows generation of carbon-centred radicals from ...

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Item type:Article
Date:2019
Institutions:Chemistry and Pharmacy > Institut für Organische Chemie > Lehrstuhl Prof. Dr. Burkhard König
Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry VI - Physical Chemistry (Solution Chemistry) > Prof. Dr. Werner Kunz
Projects:GRK 1626 Chemische Photokatalyse, KO 1537/18-1
Identification Number:
ValueType
10.1038/s41929-019-0369-5DOI
Keywords:Photocatalysis; aqueous solution
Dewey Decimal Classification:500 Science > 530 Physics
500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Partially
Item ID:40991
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